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http://hdl.handle.net/2445/185130
Title: | Designed Polynuclear Lanthanide Complexes for Quantum Information Processing |
Author: | Aguilà Avilés, David Roubeau, Olivier Aromí Bedmar, Guillem |
Keywords: | Sistemes complexos Ions Complex systems Ions |
Issue Date: | 21-Jul-2021 |
Publisher: | Royal Society of Chemistry |
Abstract: | The design of dissymmetric organic ligands featuring combinations of 1,3-diketone and 2,6-diacetylpyridine coordination pockets has been exploited to produce dinuclear and trinuclear lanthanide-based coordination compounds. These molecules exhibit two or more non-equivalent Ln ions, most remarkably enabling the access to well-defined heterolanthanide compositions. The site-selective disposition of each metal ion within the molecular entities allows the study of each centre individually as a spin-based quantum bit, affording unparalleled versatility for quantum gate design. The inherent weak interaction between the Ln ions permits the performance of multi-qubit quantum logical operations realized through their derived magnetic states, or implementing quantum-error correction protocols. The different studies performed to date on these systems are revised, showing their vast potential within spin-based quantum information processing. |
Note: | Versió postprint del document publicat a: https://doi.org/10.1039/D1DT01862K |
It is part of: | Dalton Transactions, 2021, vol. 50, p. 12045-12057 |
URI: | http://hdl.handle.net/2445/185130 |
Related resource: | https://doi.org/10.1039/D1DT01862K |
ISSN: | 1477-9226 |
Appears in Collections: | Articles publicats en revistes (Química Inorgànica i Orgànica) |
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File | Description | Size | Format | |
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715304.pdf | 1.96 MB | Adobe PDF | View/Open |
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