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http://hdl.handle.net/2445/208202
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DC Field | Value | Language |
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dc.contributor.author | Hernández-Rodríguez, Miguel A. | - |
dc.contributor.author | Brites, Carlos D. S. | - |
dc.contributor.author | Antorrena, Guillermo | - |
dc.contributor.author | Piñol, Rafael | - |
dc.contributor.author | Cases, Rafael | - |
dc.contributor.author | Pérez García, M. Lluïsa (Maria Lluïsa) | - |
dc.contributor.author | Rodrigues, Ana Mafalda Nunes | - |
dc.contributor.author | Plaza, José Antonio | - |
dc.contributor.author | Torras, Nuria | - |
dc.contributor.author | Díez, Isabel | - |
dc.contributor.author | Millán, Ángel | - |
dc.contributor.author | Carlos, Luis D. | - |
dc.date.accessioned | 2024-02-29T08:15:03Z | - |
dc.date.available | 2024-02-29T08:15:03Z | - |
dc.date.issued | 2020 | - |
dc.identifier.issn | 2195-1071 | - |
dc.identifier.uri | http://hdl.handle.net/2445/208202 | - |
dc.description.abstract | <p>The remarkable advances in molecular logic reported in the last decade</p><p>demonstrate the potential of luminescent molecules for logical operations, a</p><p>paradigm-changing concerning silicon-based electronics. Trivalent lanthanide</p><p>(Ln3+) ions, with their characteristic narrow line emissions, long-lived excited</p><p>states, and photostability under illumination, may improve the state-ofthe-</p><p>art molecular logical devices. Here, the use of monolithic silicon-based</p><p>structures incorporating Ln3+ complexes for performing logical functions is</p><p>reported. Elementary logic gates (AND, INH, and DEMUX), sequential logic</p><p>(KEYPAD LOCK), and arithmetic operations (HALF ADDER and HALF SUBTRACTOR)</p><p>exhibiting a switching ratio >60% are demonstrated for the first</p><p>time using nonwet conditions. Additionally, this is the first report showing</p><p>sequential logic and arithmetic operations combining molecular Ln3+ complexes</p><p>and physical inputs. Contrary to chemical inputs, physical inputs may</p><p>enable the future concatenation of distinct logical functions and reuse of the</p><p>logical devices, a clear step forward toward input–output homogeneity that is</p><p>precluding the integration of nowadays molecular logic devices.</p> | - |
dc.format.extent | 1 p. | - |
dc.format.mimetype | application/pdf | - |
dc.language.iso | eng | - |
dc.relation.isformatof | https://doi.org/10.1002/adom.202000312 | - |
dc.relation.ispartof | 2020, p. 2000312 | - |
dc.relation.uri | https://doi.org/10.1002/adom.202000312 | - |
dc.rights | , 2020 | - |
dc.source | Articles publicats en revistes (Farmacologia, Toxicologia i Química Terapèutica) | - |
dc.subject.classification | Fluorescència | - |
dc.subject.classification | Lligands | - |
dc.subject.other | Fluorescence | - |
dc.subject.other | Ligands | - |
dc.title | Lanthanide luminescence to mimic molecular logic and computing through physical inputs | - |
dc.type | info:eu-repo/semantics/article | - |
dc.type | info:eu-repo/semantics/ | - |
dc.identifier.idgrec | 701487 | - |
dc.date.updated | 2024-02-29T08:15:03Z | - |
dc.rights.accessRights | info:eu-repo/semantics/openAccess | - |
Appears in Collections: | Articles publicats en revistes (Farmacologia, Toxicologia i Química Terapèutica) |
Files in This Item:
File | Description | Size | Format | |
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229246.pdf | 1.2 MB | Adobe PDF | View/Open |
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