Please use this identifier to cite or link to this item:
Title: Magnetic long-range order induced by quantum ralaxation in single-molecule magnets
Author: Evangelisti, Marco
Luis Vitalla, Fernando
Mettes, F. L.
Aliaga, N. (Núria)
Aromí Bedmar, Guillem
Alonso, J. J.
Christou, G.
Jongh, L. J. de
Keywords: Materials
Propietats magnètiques
Magnetic properties and materials
Issue Date: 2004
Publisher: American Physical Society
Abstract: Can magnetic interactions between single-molecule magnets (SMMs) in a crystal establish long-range magnetic order at low temperatures deep in the quantum regime, where the only electron spin fluctuations are due to incoherent magnetic quantum tunneling (MQT)? Put inversely: can MQT provide the temperature dependent fluctuations needed to destroy the ordered state above some finite Tc, although it should basically itself be a T-independent process? Our experiments on two novel Mn4 SMMs provide a positive answer to the above, showing at the same time that MQT in the SMMs has to involve spin-lattice coupling at a relaxation rate equaling that predicted and observed recently for nuclear-spin-mediated quantum relaxation.
Note: Reproducció digital del document proporcionada per PROLA i
It is part of: Physical Review Letters, 2004, vol. 93, núm. 11, p. 117202-1-117202-4
Related resource:
ISSN: 0031-9007
Appears in Collections:Articles publicats en revistes (Química Inorgànica i Orgànica)

Files in This Item:
File Description SizeFormat 
532927.pdf278.1 kBAdobe PDFView/Open

Items in DSpace are protected by copyright, with all rights reserved, unless otherwise indicated.