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http://hdl.handle.net/2445/200464
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DC Field | Value | Language |
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dc.contributor.author | Fernández, Berta | - |
dc.contributor.author | Pi Pericay, Martí | - |
dc.contributor.author | De Lara-Castells, Maria Pilar | - |
dc.date.accessioned | 2023-07-07T14:49:40Z | - |
dc.date.available | 2023-07-07T14:49:40Z | - |
dc.date.issued | 2023-06-02 | - |
dc.identifier.issn | 1463-9076 | - |
dc.identifier.uri | http://hdl.handle.net/2445/200464 | - |
dc.description.abstract | Experimental and theoretical work has delivered evidence of the helium nanodroplet-mediated synthesis and soft-landing of metal nanoparticles, nanowires, clusters, and single atoms on solid sup- ports. Recent experimental advances have allowed the formation of charged metal clusters into multiply charged helium nanodroplets. The impact of the charge of immersed metal species in helium nanodroplet-mediated surface deposition is proved by considering silver atoms and cations at zero-temperature graphene as the support. By combining high-level ab initio intermolecular inter- action theory with a full quantum description of the superfluid helium nanodroplet motion, evidence is presented that the fundamental mechanism of soft-deposition is preserved in spite of the much stronger interaction of charged species with surfaces, with high-density fluctuations in the helium droplet playing an essential role in braking them. Corroboration is also presented that the soft- landing becomes favored as the helium nanodroplet size increases. | - |
dc.format.extent | 8 p. | - |
dc.format.mimetype | application/pdf | - |
dc.language.iso | eng | - |
dc.publisher | Royal Society of Chemistry | - |
dc.relation.isformatof | Reproducció del document publicat a: https://doi.org/10.1039/d3cp01303k | - |
dc.relation.ispartof | Physical Chemistry Chemical Physics, 2023, vol. 25, p. 16699-16706 | - |
dc.relation.uri | https://doi.org/10.1039/d3cp01303k | - |
dc.rights | cc-by-nc (c) Fernández, Berta et al., 2023 | - |
dc.rights.uri | http://creativecommons.org/licenses/by-nc/3.0/es/ | * |
dc.source | Articles publicats en revistes (Física Quàntica i Astrofísica) | - |
dc.subject.classification | Superfluïdesa | - |
dc.subject.classification | Heli | - |
dc.subject.classification | Nanopartícules | - |
dc.subject.other | Superfluidity | - |
dc.subject.other | Helium | - |
dc.subject.other | Nanoparticles | - |
dc.title | Superfluid helium droplet-mediated surface-deposition of neutral and charged silver atomic species. | - |
dc.type | info:eu-repo/semantics/article | - |
dc.type | info:eu-repo/semantics/publishedVersion | - |
dc.identifier.idgrec | 737215 | - |
dc.date.updated | 2023-07-07T14:49:40Z | - |
dc.rights.accessRights | info:eu-repo/semantics/openAccess | - |
Appears in Collections: | Articles publicats en revistes (Institut de Nanociència i Nanotecnologia (IN2UB)) Articles publicats en revistes (Física Quàntica i Astrofísica) |
Files in This Item:
File | Description | Size | Format | |
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737215.pdf | 1.11 MB | Adobe PDF | View/Open |
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