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http://hdl.handle.net/2445/133725
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DC Field | Value | Language |
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dc.contributor.author | Xu, Limei | - |
dc.contributor.author | Buldyrev, V. S. (Vladimir Sergeevich) | - |
dc.contributor.author | Stanley, H. Eugene (Harry Eugene), 1941- | - |
dc.contributor.author | Franzese, Giancarlo | - |
dc.date.accessioned | 2019-05-22T14:34:43Z | - |
dc.date.available | 2019-05-22T14:34:43Z | - |
dc.date.issued | 2012-08-27 | - |
dc.identifier.issn | 0031-9007 | - |
dc.identifier.uri | http://hdl.handle.net/2445/133725 | - |
dc.description.abstract | Several scenarios exist for the protein crystallization and aggregation in solutions near a metastable fluid-fluid phase separation below the solubility line. Based on computations, it was proposed that the fluid-fluid critical point enhances the crystallization rate by many orders of magnitude, while, based on experiments, it was proposed that the fluid-fluid spinodal controls the crystallization rate. Using molecular dynamic simulations for an isotropic model with sticky interaction, we show that neither of these scenarios adequately describes the crystallization mechanism near a metastable fluid-fluid phase separation. We find that the emergence of the high-density fluid inside the spinodal drastically enhances the crystal nucleation in the subcritical region following Ostwald's rule of stages. | - |
dc.format.extent | 5 p. | - |
dc.format.mimetype | application/pdf | - |
dc.language.iso | eng | - |
dc.publisher | American Physical Society | - |
dc.relation.isformatof | Reproducció del document publicat a: https://doi.org/10.1103/PhysRevLett.109.095702 | - |
dc.relation.ispartof | Physical Review Letters, 2012, vol. 109, num. 9, p. 095702 | - |
dc.relation.uri | https://doi.org/10.1103/PhysRevLett.109.095702 | - |
dc.rights | (c) American Physical Society, 2012 | - |
dc.source | Articles publicats en revistes (Física de la Matèria Condensada) | - |
dc.subject.classification | Física de partícules | - |
dc.subject.classification | Experiments | - |
dc.subject.other | Particle physics | - |
dc.subject.other | Experiments | - |
dc.title | Homogeneous Crystal Nucleation Near a Metastable Fluid-Fluid Phase Transition | - |
dc.type | info:eu-repo/semantics/article | - |
dc.type | info:eu-repo/semantics/publishedVersion | - |
dc.identifier.idgrec | 618158 | - |
dc.date.updated | 2019-05-22T14:34:43Z | - |
dc.relation.projectID | info:eu-repo/grantAgreement/EC/FP7/266737/EU//NANOTRANSKINETICS | - |
dc.rights.accessRights | info:eu-repo/semantics/openAccess | - |
Appears in Collections: | Articles publicats en revistes (Física de la Matèria Condensada) |
Files in This Item:
File | Description | Size | Format | |
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618158.pdf | 286.13 kB | Adobe PDF | View/Open |
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