Please use this identifier to cite or link to this item: http://hdl.handle.net/2445/133725
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dc.contributor.authorXu, Limei-
dc.contributor.authorBuldyrev, V. S. (Vladimir Sergeevich)-
dc.contributor.authorStanley, H. Eugene (Harry Eugene), 1941--
dc.contributor.authorFranzese, Giancarlo-
dc.date.accessioned2019-05-22T14:34:43Z-
dc.date.available2019-05-22T14:34:43Z-
dc.date.issued2012-08-27-
dc.identifier.issn0031-9007-
dc.identifier.urihttp://hdl.handle.net/2445/133725-
dc.description.abstractSeveral scenarios exist for the protein crystallization and aggregation in solutions near a metastable fluid-fluid phase separation below the solubility line. Based on computations, it was proposed that the fluid-fluid critical point enhances the crystallization rate by many orders of magnitude, while, based on experiments, it was proposed that the fluid-fluid spinodal controls the crystallization rate. Using molecular dynamic simulations for an isotropic model with sticky interaction, we show that neither of these scenarios adequately describes the crystallization mechanism near a metastable fluid-fluid phase separation. We find that the emergence of the high-density fluid inside the spinodal drastically enhances the crystal nucleation in the subcritical region following Ostwald's rule of stages.-
dc.format.extent5 p.-
dc.format.mimetypeapplication/pdf-
dc.language.isoeng-
dc.publisherAmerican Physical Society-
dc.relation.isformatofReproducció del document publicat a: https://doi.org/10.1103/PhysRevLett.109.095702-
dc.relation.ispartofPhysical Review Letters, 2012, vol. 109, num. 9, p. 095702-
dc.relation.urihttps://doi.org/10.1103/PhysRevLett.109.095702-
dc.rights(c) American Physical Society, 2012-
dc.subject.classificationFísica de partícules-
dc.subject.classificationExperiments-
dc.subject.otherParticle physics-
dc.subject.otherExperiments-
dc.titleHomogeneous Crystal Nucleation Near a Metastable Fluid-Fluid Phase Transition-
dc.typeinfo:eu-repo/semantics/article-
dc.typeinfo:eu-repo/semantics/publishedVersion-
dc.identifier.idgrec618158-
dc.date.updated2019-05-22T14:34:43Z-
dc.relation.projectIDinfo:eu-repo/grantAgreement/EC/FP7/266737/EU//NANOTRANSKINETICS-
dc.rights.accessRightsinfo:eu-repo/semantics/openAccess-
Appears in Collections:Articles publicats en revistes (Física de la Matèria Condensada)

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