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Fall-back time for photo-ionized Cs atoms attached to superfluid He-4 nanodroplets

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We have studied the dynamic evolution of a Cs atom photo-excited from 6s to 6p and 7s states on a helium droplet using time-dependent 4He-DFT simulations. Depending on the excited electronic state, the Cs impurity remains on the droplet surface or it is ejected. Upon subsequent photo-ionization of the excited Cs atom the resulting Cs+ cation may either be ejected or come back to the droplet, depending on the time delay between photo-excitation and photo-ionization. We have calculated the critical time delay separating these two different behaviors, as well as final ion velocities. These observables will be used for future comparison with planned pump-probe experiments.

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COPPENS, Francois, VON VANGEROW, Johannes, LEAL, Antonio, BARRANCO GÓMEZ, Manuel, HALBERSTADT, Nadine, MUDRICH, Marcel, PI PERICAY, Martí, STIENKEMEIER, Frank. Fall-back time for photo-ionized Cs atoms attached to superfluid He-4 nanodroplets. _European Physical Journal D_. 2019. Vol. 73, núm. 5. [consulta: 23 de gener de 2026]. ISSN: 1434-6060. [Disponible a: https://hdl.handle.net/2445/192311]

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