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Tunneling magnetoresistance in Co-ZrO2 granular thin films

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Granular films composed of well defined nanometric Co particles embedded in an insulating ZrO2 matrix were prepared by pulsed laser depositon in a wide range of Co volume concentrations 0.15 x 0.43. High-resolution transmission electron microscopy TEM showed very sharp interfaces between the crystalline particles and the amorphous matrix. Narrow particle size distributions were determined from TEM and by fitting the low-field magnetic susceptibility and isothermal magnetization in the paramagnetic regime to a distribution of Langevin functions. The magnetic particle size varies little for Co volume concentrations x 0.32 and increases as the percolation limit is approached. The tunneling magnetoresistance TMR was successfully reproduced using the Inoue-Maekawa model. The maximum value of TMR was temperatureindependent within 50–300 K, and largely increased at low T, suggesting the occurrence of higher-order tunneling processes. Consequently, the tunneling conductance and TMR in clean granular metals are dominated by the Coulomb gap and the inherent particle size distribution.

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HATTINK, Bart jan, GARCÍA DEL MURO Y SOLANS, Montserrat, KONSTANTINOVIĆ, Zorica, BATLLE GELABERT, Xavier, LABARTA, Amílcar. Tunneling magnetoresistance in Co-ZrO2 granular thin films. _Physical Review B_. 2006. Vol. 73, núm. 4, pàgs. 045418-1-045418-9. [consulta: 30 de gener de 2026]. ISSN: 0163-1829. [Disponible a: https://hdl.handle.net/2445/10648]

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