Carregant...
Miniatura

Tipus de document

Article

Versió

Versió publicada

Data de publicació

Llicència de publicació

cc-by (c) Pallara, Chiara et al., 2022
Si us plau utilitzeu sempre aquest identificador per citar o enllaçar aquest document: https://hdl.handle.net/2445/190110

Peptidomimetics designed to bind to RAS effector domain are promising cancer therapeutic compounds.

Títol de la revista

Director/Tutor

ISSN de la revista

Títol del volum

Resum

Oncogenic RAS proteins are important for driving tumour formation, and for maintenance of the transformed phenotype, and thus their relevance as a cancer therapeutic target is undeniable. We focused here on obtaining peptidomimetics, which have good pharmacological properties, to block Ras-effector interaction. Computational analysis was used to identify hot spots of RAS relevant for these interactions and to screen a library of peptidomimetics. Nine compounds were synthesized and assayed for their activity as RAS inhibitors in cultured cells. Most of them induced a reduction in ERK and AKT activation by EGF, a marker of RAS activity. The most potent inhibitor disrupted Raf and PI3K interaction with oncogenic KRAS, corroborating its mechanism of action as an inhibitor of protein-protein interactions, and thus validating our computational methodology. Most interestingly, improvement of one of the compounds allowed us to obtain a peptidomimetic that decreased the survival of pancreatic cancer cell lines harbouring oncogenic KRAS

Citació

Citació

PALLARA, Chiara, CABOT, Débora, RIVAS, Josep, BRUN, Sonia, SECO, Jesús, ABUASAKER, Baraa, TARRAGÓ CLUA, Maria teresa, JAUMOT I PIJOAN, Montserrat, PRADES, Roger, AGELL I JANÉ, Neus. Peptidomimetics designed to bind to RAS effector domain are promising cancer therapeutic compounds.. _Scientific Reports_. 2022. Vol. 22, núm. 12, pàgs. 15810. [consulta: 21 de gener de 2026]. ISSN: 2045-2322. [Disponible a: https://hdl.handle.net/2445/190110]

Exportar metadades

JSON - METS

Compartir registre