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Si us plau utilitzeu sempre aquest identificador per citar o enllaçar aquest document: https://hdl.handle.net/2445/148842
Spatiotemporal control of cargo delivery performed by programmable self-propelled Janus droplets
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Self-propelled droplets capable of transporting cargo to specific target locations are desired tools for many future applications. Here we propose a class of active droplets with programmable delivery time that are attracted or repelled by certain obstacle geometries. These droplets consist of a water/ethanol mixture and are dispersed in an oil/surfactant solution. Owing to a mass exchange between fluid phases during self-propulsion, the initially homogeneous droplets spontaneously de-mix and evolve into characteristic Janus droplets. Cargo molecules, like DNA, can be separated into the trailing ethanol-rich droplet and are carried to their target location 'like in a backpack'. The delayed onset of phase separation provides a handle to control the time frame of delivery, while long-ranged hydrodynamic interactions and short-ranged wetting forces are exploited to achieve the desired spatial specificity with respect to obstacle geometry and surface chemistry.
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LI, Menglin, BRINKMANN, Martin, PAGONABARRAGA MORA, Ignacio, SEEMAN, Ralf, FLEURY, Jean-baptiste. Spatiotemporal control of cargo delivery performed by programmable self-propelled Janus droplets. _Communications Physics_. 2018. Vol. 1, núm. 23. [consulta: 25 de gener de 2026]. [Disponible a: https://hdl.handle.net/2445/148842]