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cc by-nc-nd (c) Elsevier B.V., 2017
Si us plau utilitzeu sempre aquest identificador per citar o enllaçar aquest document: https://hdl.handle.net/2445/110939

2-picolylamine derivatization for high sensitivity detection of abscisic acid in apicomplexan blood-infecting parasites

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We have developed a new liquid chromatography-electrospray ionization tandem mass spectrometry methodology based on 2-picolylamine derivatization and positive ion mode detection for abscisic acid (ABA) identification. The selected reaction leads to the formation of an amide derivative which contains a highly active pyridyl group. The enhanced ionization allows for a 700-fold increase over commonly monitored unmodified ABA, which in turn leads to excellent limits of detection and quantification values of 0.03 and 0.15ngmL-1, respectively. This method has been validated in the highly complex matrix of a red blood cell extract. In spite of the high sensitivity achieved, ABA could not be detected in Plasmodium falciparum-infected red blood cells, suggesting that, if present, it will be found either in ultratrace amounts or as brief bursts at defined time points within the intraerythrocytic cycle and/or in the form of a biosynthetic analogue.

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MOLES MELER, Ernest, MARCOS, Josep, IMPERIAL RÓDENAS, Santiago, POZO, Oscar j., FERNÀNDEZ BUSQUETS, Xavier. 2-picolylamine derivatization for high sensitivity detection of
                abscisic acid in apicomplexan blood-infecting parasites. _Talanta_. 2017. Vol. 168, núm. 130-135. [consulta: 31 de gener de 2026]. ISSN: 0039-9140. [Disponible a: https://hdl.handle.net/2445/110939]

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