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2021-07-21

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Designed Polynuclear Lanthanide Complexes for Quantum Information Processing

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https://doi.org/10.1039/D1DT01862K

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The design of dissymmetric organic ligands featuring combinations of 1,3-diketone and 2,6-diacetylpyridine coordination pockets has been exploited to produce dinuclear and trinuclear lanthanide-based coordination compounds. These molecules exhibit two or more non-equivalent Ln ions, most remarkably enabling the access to well-defined heterolanthanide compositions. The site-selective disposition of each metal ion within the molecular entities allows the study of each centre individually as a spin-based quantum bit, affording unparalleled versatility for quantum gate design. The inherent weak interaction between the Ln ions permits the performance of multi-qubit quantum logical operations realized through their derived magnetic states, or implementing quantum-error correction protocols. The different studies performed to date on these systems are revised, showing their vast potential within spin-based quantum information processing.

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Sistemes complexos, Ions

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Complex systems, Ions

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Articles publicats en revistes (Química Inorgànica i Orgànica)

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AGUILÀ AVILÉS, David, ROUBEAU, Olivier and AROMÍ BEDMAR, Guillem. Designed Polynuclear Lanthanide Complexes for Quantum Information Processing. Dalton Transactions. 2021. Vol. 50, num. 12045-12057. ISSN 1477-9226. [consulted: 30 of May of 2026]. Available at: https://hdl.handle.net/2445/185130

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