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cc-by (c) Mautner, Franz A. et al., 2022
Si us plau utilitzeu sempre aquest identificador per citar o enllaçar aquest document: https://hdl.handle.net/2445/192045

Magnetic and Luminescence Properties of 8-Coordinated Pyridyl Adducts of Samarium(III) Complexes Containing 4,4,4-Trifluoro-1-(naphthalen-2-yl)-1,3-butanedionate

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A novel series of polypyridyl adducts, [Sm(ntfa)3(NN)] (2-4), with ntfa = 4,4,4-trifluoro-1-(naphthalen-2-yl)-1,3-butanedionate, NN = 2,2′-bipyridine (bipy), 4,4′-dimethyl-2,2′-bipyridine (4,4′-Me2bipy), and 5,5′-dimethyl-2,2′-bipyridine (5,5′-Me2bipy) were synthesized from the precursor complex [Sm(ntfa)3(MeOH)2] (1) and the corresponding pyridyl ligands. Single X-ray crystallography showed that the complexes displayed 8-coordinated geometry. The solid pyridyl adducts 2-4 exhibited emission of luminescence in the NIR and visible regions with close quantum yields (QY = 0.20-0.25%). The magnetic data of 1-4 showed larger values than those expected for magnetically noncoupled Sm(III) complexes in the 6H5/2 ground state, with no saturation on the applied high magnetic field static at a temperature of 2 K.

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MAUTNER, Franz a., BIERBAUMER, Florian, VICENTE CASTILLO, Ramón, SPEED CASTRO, Saskia, TUBAU RIBOT, Ànnia, FISCHER, Roland c., MASSOUD, Salah s.. Magnetic and Luminescence Properties of 8-Coordinated Pyridyl Adducts of Samarium(III) Complexes Containing 4,4,4-Trifluoro-1-(naphthalen-2-yl)-1,3-butanedionate. _Magnetochemistry_. 2022. Vol. 8, núm. 72. [consulta: 7 de febrer de 2026]. ISSN: 2312-7481. [Disponible a: https://hdl.handle.net/2445/192045]

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