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From isodesmic to highly cooperative: Reverting the supramolecular polymerization mechanism in water by fine monomer design
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Two structurally-similar discotic molecules able to self-assemble in water, forming supramolecular fibers, are reported. While both self-assembled polymers are indistinguishable from a morphological point-of-view, a dramatic change in their polymerization mechanism is observed (i.e., one self-assemble via an isodesmic mechanism, while the other shows one of the highest cooperativity values).
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CASELLAS, Nicolas M., et al. From isodesmic to highly cooperative: Reverting the supramolecular polymerization mechanism in water by fine monomer design. Chemical Communications. 2018. Vol. 54, num. 33, pags. 4112-4115. [consulted: 9 of October of 2026]. Available at: https://hdl.handle.net/2445/127393