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cc-by-nc-nd (c) Elsevier B.V., 2016
Si us plau utilitzeu sempre aquest identificador per citar o enllaçar aquest document: https://hdl.handle.net/2445/128326

Comparison of the thermal decomposition processes of several aminoalcohol-based ZnO inks with one containing ethanolamine

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Four inks for the production of ZnO semiconducting films have been prepared with zinc acetate dihy-drate as precursor salt and one among the following aminoalcohols: aminopropanol (APr), aminomethylbutanol (AMB), aminophenol (APh) and aminobenzyl alcohol (AB) as stabilizing agent. Their thermaldecomposition process has been analyzed in situ by thermogravimetric analysis (TGA), differential scan-ning calorimetry (DSC) and evolved gas analysis (EGA), whereas the solid product has been analysedex-situ by X-ray diffraction (XRD) and infrared spectroscopy (IR). Although, except for the APh ink, crys-talline ZnO is already obtained at 300◦C, the films contain an organic residue that evolves at highertemperature in the form of a large variety of nitrogen-containing cyclic compounds. The results indicatethat APr can be a better stabilizing agent than ethanolamine (EA). It gives larger ZnO crystal sizes withsimilar carbon content. However, a common drawback of all the amino stabilizers (EA included) is thatnitrogen atoms have not been completely removed from the ZnO film at the highest temperature of ourexperiments (600◦C).

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GÓMEZ NÚÑEZ, Alberto, ROURA GRABULOSA, Pere, LÓPEZ MARTÍNEZ, Ma. concepción, VILÀ I ARBONÈS, Anna maria. Comparison of the thermal decomposition processes of several aminoalcohol-based ZnO inks with one containing ethanolamine. _Applied Surface Science_. 2016. Vol. 381, núm. 48-53. [consulta: 22 de gener de 2026]. ISSN: 0169-4332. [Disponible a: https://hdl.handle.net/2445/128326]

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