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2021_ChemRev_Peptide_KumarM.pdf (18.19 MB)

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2021-09-14

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cc by-nc-nd (c) Sheehan, Fahmeed et al, 2021
Si us plau utilitzeu sempre aquest identificador per citar o enllaçar aquest document: https://hdl.handle.net/2445/199367

Peptide-Based Supramolecular Systems Chemistry

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Recurs relacionat

https://doi.org/10.1021/acs.chemrev.1c00089

Resum

Peptide-based supramolecular systems chemistry seeks to mimic the ability of life forms to use conserved sets of building blocks and chemical reactions to achieve a bewildering array of functions. Building on the design principles for short peptide-based nanomaterials with properties, such as self-assembly, recognition, catalysis, and actuation, are increasingly available. Peptide-based supramolecular systems chemistry is starting to address the far greater challenge of systems-level design to access complex functions that emerge when multiple reactions and interactions are coordinated and integrated. We discuss key features relevant to systems-level design, including regulating supramolecular order and disorder, development of active and adaptive systems by considering kinetic and thermodynamic design aspects and combinatorial dynamic covalent and noncovalent interactions. Finally, we discuss how structural and dynamic design concepts, including preorganization and induced fit, are critical to the ability to develop adaptive materials with adaptive and tunable photonic, electronic, and catalytic properties. Finally, we highlight examples where multiple features are combined, resulting in chemical systems and materials that display adaptive properties that cannot be achieved without this level of integration.

Matèries

Pèptids, Termodinàmica

Matèries (anglès)

Peptides, Thermodynamics

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Articles publicats en revistes (Institut de Bioenginyeria de Catalunya (IBEC))

Citació

SHEEHAN, Fahmeed, SEMENTA, Deborah, JAIN, Ankit, KUMAR, Mohit, TAYARANI-NAJJARAN, Mona, KROISS, Daniela, ULIJN, Rein v.. Peptide-Based Supramolecular Systems Chemistry. _Chemical Reviews_. 2021. Vol. 121, núm. 22, pàgs. 13869-13914. [consulta: 21 de gener de 2026]. ISSN: 1520-6890. [Disponible a: https://hdl.handle.net/2445/199367]

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