Redox shield enfolding a magnetic core

dc.contributor.authorKishore, Pilli V.V.
dc.contributor.authorRasamsetty, Amaleswari
dc.contributor.authorSañudo Zotes, Eva Carolina
dc.contributor.authorBaskar, Viswanathan
dc.date.accessioned2020-03-27T07:05:45Z
dc.date.available2020-03-27T07:05:45Z
dc.date.issued2015-12-23
dc.date.updated2020-03-27T07:05:46Z
dc.description.abstractFerrocenyl betadiketones were reacted with hydrated lanthanide trihalides in presence of a base to yield red color solids, whose structures were characterized by single crystal X-ray diffraction technique. Structural analysis revealed the formation of nona- and tetranuclear lanthanide oxo-hydroxo clusters [Dy9(μ4-O)2(μ3-OH)8(μ-Fca)8(Fca)8]−[HN(C2H5)3]+ (1), [Ln4(μ-OH)2(μ-OCH3)4(CH3OH)2(Fctfa)6] Ln = Yb (2), Lu (3), and [Ln4(μ-OH)2(μ-OCH3)4(CH3OH)2(Fcpfa)6] Ln = Yb (4), Lu (5). Magnetism studies revealed that 1 shows slow relaxation of magnetisation. Cyclic voltammetry studies of 1 reveal electrochemically stable quasi reversible oxidation systems whereas 2-5 showed irreversible nature.
dc.format.extent5 p.
dc.format.mimetypeapplication/pdf
dc.identifier.idgrec662178
dc.identifier.issn0277-5387
dc.identifier.urihttps://hdl.handle.net/2445/154124
dc.language.isoeng
dc.publisherElsevier Ltd
dc.relation.isformatofVersió postprint del document publicat a: https://doi.org/10.1016/j.poly.2015.10.017
dc.relation.ispartofPolyhedron, 2015, vol. 102, p. 361-365
dc.relation.urihttps://doi.org/10.1016/j.poly.2015.10.017
dc.rightscc-by-nc-nd (c) Elsevier Ltd, 2015
dc.rights.accessRightsinfo:eu-repo/semantics/openAccess
dc.rights.urihttp://creativecommons.org/licenses/by-nc-nd/3.0/es
dc.sourceArticles publicats en revistes (Química Inorgànica i Orgànica)
dc.subject.classificationTerres rares
dc.subject.classificationImants
dc.subject.classificationDifracció de raigs X
dc.subject.otherRare earths
dc.subject.otherMagnets
dc.subject.otherX-rays diffraction
dc.titleRedox shield enfolding a magnetic core
dc.typeinfo:eu-repo/semantics/article
dc.typeinfo:eu-repo/semantics/acceptedVersion

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